First study of the ro-vibrational structure of the g-symmetry vibrational states of C2D4 from the analysis of hot bands: The v7+v10-v10 and v10+v12-v10 bands

Bibliographic Details
Parent link:Journal of Quantitative Spectroscopy and Radiative Transfer
Vol. 187.— 2017.— [P. 178–189]
Corporate Author: Национальный исследовательский Томский политехнический университет (ТПУ) Физико-технический институт (ФТИ) Кафедра общей физики (ОФ)
Other Authors: Ulenekov (Ulenikov) O. N. Oleg Nikolaevich, Gromova O. V. Olga Vasilievna, Bekhtereva E. S. Elena Sergeevna, Fomchenko A. L. Anna Leonidovna, Sydow C., Maul C. Christof, Bauerecker S. Sigurd
Summary:Title screen
The two strongest absorption "hot" bands of C2D4, ν7+ν10−ν10 and ν10+ν12−ν10 were analyzed for the first time on the basis of high resolution infrared spectra recorded with a Bruker high resolution Fourier transform spectrometer. About 740 and 550 transitions (233 and 174 upper state ro-vibrational energy values) with Jmax.=25, Ka,max =18 and Jmax.=20, Ka,max =10 for the bands ν7+ν10−ν10 and ν10+ν12−ν10 were assigned. The obtained upper ro-vibrational energies were used then in the weighted fit of parameters of the effective Hamiltonian which takes into account resonance interactions between the vibrational states (v7=v10=1) and (v10=v12=1), on the one hand, and eight other closely located vibrational states, on the other hand. A set of 46 varied parameters was obtained from the fit, which reproduces the initial experimental data with the rms deviation of 2.5 x 10[-4] cm[-1] and which is close to experimental uncertainties.
Режим доступа: по договору с организацией-держателем ресурса
Published: 2017
Subjects:
Online Access:http://dx.doi.org/10.1016/j.jqsrt.2016.09.014
Format: Electronic Book Chapter
KOHA link:https://koha.lib.tpu.ru/cgi-bin/koha/opac-detail.pl?biblionumber=653234