Novel Biocompatible Magnetoelectric MnFe2O4 Core@BCZT Shell Nano–Hetero-Structures with Efficient Catalytic Performance; Small; Vol. 19, iss. 42

Bibliographische Detailangaben
Parent link:Small.— .— Washington: John Wiley and Sons Ltd.
Vol. 19, iss. 42.— 2023.— Article number 2302808, 17 p.
Weitere Verfasser: Chernozem R. V. Roman Viktorovich, Urakova A. O. Alina Olegovna, Chernozem P. V. Polina Viktorovna, Koptsev D. A. Danila Andreevich, Mukhortova Yu. R. Yulia Ruslanovna, Grubova I. Yu. Irina Yurievna, Vagner D. V. Dmitry Viktorovich, Gerasimov E. Yu. Evgeny Yurjevich, Surmeneva M. A. Maria Alexandrovna, Kholkin A. L. Andrei Leonidovich, Surmenev R. A. Roman Anatolievich
Zusammenfassung:Title screen
Magnetoelectric (ME) small-scale robotic devices attract great interest from the scientific community due to their unique properties for biomedical applications. Here, novel ME nano hetero-structures based on the biocompatible magnetostrictive MnFe2O4 (MFO) and ferroelectric Ba0.85Ca0.15Zr0.1Ti0.9O3 (BCZT) are developed solely via the hydrothermal method for the first time. An increase in the temperature and duration of the hydrothermal synthesis results in increasing the size, improving the purity, and inducing morphology changes of MFO nanoparticles (NPs). A successful formation of a thin epitaxial BCZT-shell with a 2–5 nm thickness is confirmed on the MFO NPs (77 ± 14 nm) preliminarily treated with oleic acid (OA) or polyvinylpyrrolidone (PVP), whereas no shell is revealed on the surface of pristine MFO NPs. High magnetization is revealed for the developed ME NPs based on PVP- and OA-functionalized MFO NPs (18.68 ± 0.13 and 20.74 ± 0.22 emu g−1, respectively). Moreover, ME NPs demonstrate 95% degradation of a model pollutant Rhodamine B within 2.5 h under an external AC magnetic field (150 mT, 100 Hz). Thus, the developed biocompatible core–shell ME NPs of MFO and BCZT can be considered as a promising tool for non-invasive biomedical applications, environmental remediation, and hydrogen generation for renewable energy sources
Текстовый файл
AM_Agreement
Sprache:Englisch
Veröffentlicht: 2023
Schlagworte:
Online-Zugang:https://doi.org/10.1002/smll.202302808
Format: Elektronisch Buchkapitel
KOHA link:https://koha.lib.tpu.ru/cgi-bin/koha/opac-detail.pl?biblionumber=685016

MARC

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330 |a Magnetoelectric (ME) small-scale robotic devices attract great interest from the scientific community due to their unique properties for biomedical applications. Here, novel ME nano hetero-structures based on the biocompatible magnetostrictive MnFe2O4 (MFO) and ferroelectric Ba0.85Ca0.15Zr0.1Ti0.9O3 (BCZT) are developed solely via the hydrothermal method for the first time. An increase in the temperature and duration of the hydrothermal synthesis results in increasing the size, improving the purity, and inducing morphology changes of MFO nanoparticles (NPs). A successful formation of a thin epitaxial BCZT-shell with a 2–5 nm thickness is confirmed on the MFO NPs (77 ± 14 nm) preliminarily treated with oleic acid (OA) or polyvinylpyrrolidone (PVP), whereas no shell is revealed on the surface of pristine MFO NPs. High magnetization is revealed for the developed ME NPs based on PVP- and OA-functionalized MFO NPs (18.68 ± 0.13 and 20.74 ± 0.22 emu g−1, respectively). Moreover, ME NPs demonstrate 95% degradation of a model pollutant Rhodamine B within 2.5 h under an external AC magnetic field (150 mT, 100 Hz). Thus, the developed biocompatible core–shell ME NPs of MFO and BCZT can be considered as a promising tool for non-invasive biomedical applications, environmental remediation, and hydrogen generation for renewable energy sources 
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701 1 |a Chernozem  |b R. V.  |c physicist  |c Associate Professor of Tomsk Polytechnic University  |f 1992-  |g Roman Viktorovich  |9 19499 
701 1 |a Urakova  |b A. O.  |c specialist in the field of material science  |c Laboratory assistant of Tomsk Polytechnic University  |f 2002-  |g Alina Olegovna  |9 88596 
701 1 |a Chernozem  |b P. V.  |c specialist in the field of informatics and computer technology  |c Research Engineer of Tomsk Polytechnic University  |f 1997-  |g Polina Viktorovna  |9 22733 
701 1 |a Koptsev  |b D. A.  |c specialist in the field of material science  |c Laboratory assistant of Tomsk Polytechnic University  |f 2003-  |g Danila Andreevich  |9 88597 
701 1 |a Mukhortova  |b Yu. R.  |c Chemical engineer  |c Engineer of Tomsk Polytechnic University  |f 1976-  |g Yulia Ruslanovna  |9 22264 
701 1 |a Grubova  |b I. Yu.  |c physicist  |c engineer-researcher of Tomsk Polytechnic Universit  |f 1989-  |g Irina Yurievna  |9 16573 
701 1 |a Vagner  |b D. V.  |g Dmitry Viktorovich 
701 1 |a Gerasimov  |b E. Yu.  |g Evgeny Yurjevich 
701 1 |a Surmeneva  |b M. A.  |c specialist in the field of material science  |c engineer-researcher of Tomsk Polytechnic University, Associate Scientist  |f 1984-  |g Maria Alexandrovna  |9 15966 
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