Improved Theory of the Effective Dipole Moments and Absolute Line Strengths of the XY2 Asymmetric Top Molecules in the X2B1 Doublet Electronic States; International Journal of Molecular Sciences; Vol. 24, iss. 16

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Parent link:International Journal of Molecular Sciences.— .— Basel: MDPI AG
Vol. 24, iss. 16.— 2023.— Article number 12734, 19 p.
Další autoři: Ulenekov (Ulenikov) O. N. Oleg Nikolaevich, Bekhtereva E. S. Elena Sergeevna, Gromova O. V. Olga Vasilievna, Kakaulin A. N. Aleksey Nikolaevich, Sydow Ch. Christian, Bauerecker (Bauerekker) Z. (S.) H. Zigurd (Sigurd) Hermann
Shrnutí:Title screen
A new effective dipole moment model for the XY2 (𝐶2𝑣C2v−symmetry) molecule in a doublet electronic state is derived that includes (as special cases) all currently known models of effective dipole moments for such types of molecules, and allows us to take into account the influence of spin–rotation interactions on the effective dipole moment operator that were not considered in the preceding studies. Necessary for the analysis of absolute line strengths, the matrix elements of this dipole moment operator are derived. A comparison with the previous analog models is made and discussed. The efficiency of the obtained results is illustrated, which have been applied to a set of the “forbidden” Δ𝐾𝑎=2ΔKa=2 transitions of the 𝜈3ν3 band of the OClO free radical molecule
Текстовый файл
Jazyk:angličtina
Vydáno: 2023
Témata:
On-line přístup:http://earchive.tpu.ru/handle/11683/132518
https://doi.org/10.3390/ijms241612734
Médium: Elektronický zdroj Kapitola
KOHA link:https://koha.lib.tpu.ru/cgi-bin/koha/opac-detail.pl?biblionumber=680446

MARC

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330 |a A new effective dipole moment model for the XY2 (2C2v−symmetry) molecule in a doublet electronic state is derived that includes (as special cases) all currently known models of effective dipole moments for such types of molecules, and allows us to take into account the influence of spin–rotation interactions on the effective dipole moment operator that were not considered in the preceding studies. Necessary for the analysis of absolute line strengths, the matrix elements of this dipole moment operator are derived. A comparison with the previous analog models is made and discussed. The efficiency of the obtained results is illustrated, which have been applied to a set of the “forbidden” Δ=2ΔKa=2 transitions of the 3ν3 band of the OClO free radical molecule 
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463 1 |t Vol. 24, iss. 16  |v Article number 12734, 19 p.  |d 2023 
610 1 |a asymmetric top molecules in non-singlet electronic states 
610 1 |a spin–rotation interactions 
610 1 |a absolute line strengths 
610 1 |a effective dipole moment operator 
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701 1 |a Ulenekov (Ulenikov)  |b O. N.  |c physicist  |c Professor of Tomsk Polytechnic University, Doctor of physical and mathematical sciences  |f 1949-  |g Oleg Nikolaevich  |9 17837 
701 1 |a Bekhtereva  |b E. S.  |c physicist  |c Professor of Tomsk Polytechnic University, Doctor of physical and mathematical sciences  |f 1974-  |g Elena Sergeevna  |9 17851 
701 1 |a Gromova  |b O. V.  |c physicist  |c Professor of Tomsk Polytechnic University, Candidate of physical and mathematical sciences  |f 1982-  |g Olga Vasilievna  |9 17839 
701 1 |a Kakaulin  |b A. N.  |c physicist  |c Technician of Tomsk Polytechnic University  |f 1998-  |g Aleksey Nikolaevich  |9 22804 
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701 1 |a Bauerecker (Bauerekker)  |b Z. (S.) H.  |c physicist  |c Junior researcher at Tomsk Polytechnic University  |f 1960-  |g Zigurd (Sigurd) Hermann  |9 20429 
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