Submillimeter wave spectrum of methylene chloride, 12CH235Cl2, 12CH235Cl37Cl and 12CH237Cl2 up to 1.1 THz

Dettagli Bibliografici
Parent link:Journal of Quantitative Spectroscopy and Radiative Transfer.— .— Amsterdam: Elsevier Science Publishing Company Inc.
Vol. 319.— 2024.— 108962, 14 p.
Ente Autore: National Research Tomsk Polytechnic University (570)
Altri autori: Ulenekov (Ulenikov) O. N. Oleg Nikolaevich, Gromova O. V. Olga Vasilievna, Bekhtereva E. S. Elena Sergeevna, Muller H. S. P. Holger, Margules L. B. Laurent
Riassunto:High resolution spectra of methylene chloride in natural abundance are recorded in wide spectral regions from 0.075 up to 1.090 THz. The 5095 multiplet center frequencies with the value of quantum number Jmax=107 and Kamax=20 were assigned to the 12CH235Cl2 species. A weighed fit of the experimental data allowed us to obtain a set of 20 rotational and centrifugal distortion parameters which reproduce the initial experimental data with the drms=19 kHz in the whole region. Comparison with the literature values from microwave and from far infrared measurements is made. An analogous analysis was carried out for the 12CH235Cl37Cl and 12CH237Cl2 species for which 4561 and 2465 transitions with Jmax=100, Kamax=19 and Jmax=88, Kamax=19 where assigned and analyzed. Sets of 20 fitted effective Hamiltonian parameters of 12CH235Cl37Cl and 15 fitted parameters of 12CH237Cl2 reproduce the assigned experimental transitions of the latter two isotopologues with the drms=20 kHz and drms=19 kHz, respectively and considerably improve the calculated line positions up to 1.1 THz in comparison with previous parameters.
Текстовый файл
AM_Agreement
Lingua:inglese
Pubblicazione: 2024
Soggetti:
Accesso online:https://doi.org/10.1016/j.jqsrt.2024.108962
Natura: Elettronico Capitolo di libro
KOHA link:https://koha.lib.tpu.ru/cgi-bin/koha/opac-detail.pl?biblionumber=674298

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200 |a Submillimeter wave spectrum of methylene chloride, 12CH235Cl2, 12CH235Cl37Cl and 12CH237Cl2 up to 1.1 THz  |f O. N. Ulenikov, O. V. Gromova, E. S. Bekhtereva [et al.] 
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330 |a High resolution spectra of methylene chloride in natural abundance are recorded in wide spectral regions from 0.075 up to 1.090 THz. The 5095 multiplet center frequencies with the value of quantum number Jmax=107 and Kamax=20 were assigned to the 12CH235Cl2 species. A weighed fit of the experimental data allowed us to obtain a set of 20 rotational and centrifugal distortion parameters which reproduce the initial experimental data with the drms=19 kHz in the whole region. Comparison with the literature values from microwave and from far infrared measurements is made. An analogous analysis was carried out for the 12CH235Cl37Cl and 12CH237Cl2 species for which 4561 and 2465 transitions with Jmax=100, Kamax=19 and Jmax=88, Kamax=19 where assigned and analyzed. Sets of 20 fitted effective Hamiltonian parameters of 12CH235Cl37Cl and 15 fitted parameters of 12CH237Cl2 reproduce the assigned experimental transitions of the latter two isotopologues with the drms=20 kHz and drms=19 kHz, respectively and considerably improve the calculated line positions up to 1.1 THz in comparison with previous parameters. 
336 |a Текстовый файл 
371 0 |a AM_Agreement 
461 1 |t Journal of Quantitative Spectroscopy and Radiative Transfer  |c Amsterdam  |n Elsevier Science Publishing Company Inc. 
463 1 |t Vol. 319  |v 108962, 14 p.  |d 2024 
610 1 |a электронный ресурс 
610 1 |a труды учёных ТПУ 
610 1 |a Quadrupole splitting in methylene chloride 
610 1 |a Isotopologues of methylene chloride 
610 1 |a Rotational and centrifugal distortion parameters 
701 1 |a Ulenekov (Ulenikov)  |b O. N.  |c physicist  |c Professor of Tomsk Polytechnic University, Doctor of physical and mathematical sciences  |f 1949-  |g Oleg Nikolaevich  |9 17837 
701 1 |a Gromova  |b O. V.  |c physicist  |c Professor of Tomsk Polytechnic University, Candidate of physical and mathematical sciences  |f 1982-  |g Olga Vasilievna  |9 17839 
701 1 |a Bekhtereva  |b E. S.  |c physicist  |c Professor of Tomsk Polytechnic University, Doctor of physical and mathematical sciences  |f 1974-  |g Elena Sergeevna  |9 17851 
701 1 |a Muller  |b H. S. P.  |g Holger 
701 1 |a Margules  |b L. B.  |g Laurent 
712 0 2 |a National Research Tomsk Polytechnic University  |c (2009- )  |9 27197  |4 570 
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