In Vitro Biodegradation of a-C:H:SiOx Films on Ti-6Al-4V Alloy

Détails bibliographiques
Parent link:Materials
Vol. 15, iss. 12.— 2022.— [4239, 17 p.]
Collectivité auteur: Национальный исследовательский Томский политехнический университет Исследовательская школа химических и биомедицинских технологий
Autres auteurs: Grenaderov A. S. Aleksandr Sergeevich, Solovyev A. Andrey, Oskomov K. V. Konstantin Vladimirovich, Porokhova E. Ekaterina, Brazovsky (Brazovskii) K. S. Konstantin Stanislavovich, Gorokhova A. V. Anna Viktorovna, Nasibov T. Temur, Litvinova L. Larisa, Khlusov I. A. Igor Albertovich
Résumé:Title screen
This paper focuses mainly on the in vitro study of a five-week biodegradation of a-C:H:SiOx films of different thickness, obtained by plasma-assisted chemical vapor deposition onto Ti-6Al-4V alloy substrate using its pulsed bipolar biasing. In vitro immersion of a-C:H:SiOx films in a solution of 0.9% NaCl was used. It is shown how the a-C:H:SiOx film thickness (0.5-3 µm) affects the surface morphology, adhesive strength, and Na+ and Cl− precipitation on the film surface from the NaCl solution. With increasing film thickness, the roughness indices are reducing a little. The adhesive strength of the a-C:H:SiOx films to metal substrate corresponds to quality HF1 (0.5 µm in thickness) and HF2-HF3 (1.5-3 µm in thickness) of the Rockwell hardness test (VDI 3198) that defines strong interfacial adhesion and is usually applied in practice. The morphometric analysis of the film surface shows that on a-C:H:SiOx-coated Ti-6Al-4V alloy surface, the area occupied by the grains of sodium chloride is lower than on the uncoated surface. The reduction in the ion precipitation from 0.9% NaCl onto the film surface depended on the elemental composition of the surface layer conditioned by the thickness growth of the a-C:H:SiOx film. Based on the results of energy dispersive X-ray spectroscopy, the multiple regression equations are suggested to explain the effect of the elemental composition of the a-C:H:SiOx film on the decreased Na+ and Cl− precipitation. As a result, the a-C:H:SiOx films successfully combine good adhesion strength and rare ion precipitation and thus are rather promising for medical applications on cardiovascular stents and/or friction parts of heart pumps.
Langue:anglais
Publié: 2022
Sujets:
Accès en ligne:https://doi.org/10.3390/ma15124239
Format: Électronique Chapitre de livre
KOHA link:https://koha.lib.tpu.ru/cgi-bin/koha/opac-detail.pl?biblionumber=668245

MARC

LEADER 00000naa0a2200000 4500
001 668245
005 20250314163239.0
035 |a (RuTPU)RU\TPU\network\39469 
035 |a RU\TPU\network\39390 
090 |a 668245 
100 |a 20220706d2022 k||y0rusy50 ba 
101 0 |a eng 
135 |a drcn ---uucaa 
181 0 |a i  
182 0 |a b 
200 1 |a In Vitro Biodegradation of a-C:H:SiOx Films on Ti-6Al-4V Alloy  |f A. S. Grenaderov, A. Solovyev, K. V. Oskomov [et al.] 
203 |a Text  |c electronic 
300 |a Title screen 
320 |a [References: 55 tit.] 
330 |a This paper focuses mainly on the in vitro study of a five-week biodegradation of a-C:H:SiOx films of different thickness, obtained by plasma-assisted chemical vapor deposition onto Ti-6Al-4V alloy substrate using its pulsed bipolar biasing. In vitro immersion of a-C:H:SiOx films in a solution of 0.9% NaCl was used. It is shown how the a-C:H:SiOx film thickness (0.5-3 µm) affects the surface morphology, adhesive strength, and Na+ and Cl− precipitation on the film surface from the NaCl solution. With increasing film thickness, the roughness indices are reducing a little. The adhesive strength of the a-C:H:SiOx films to metal substrate corresponds to quality HF1 (0.5 µm in thickness) and HF2-HF3 (1.5-3 µm in thickness) of the Rockwell hardness test (VDI 3198) that defines strong interfacial adhesion and is usually applied in practice. The morphometric analysis of the film surface shows that on a-C:H:SiOx-coated Ti-6Al-4V alloy surface, the area occupied by the grains of sodium chloride is lower than on the uncoated surface. The reduction in the ion precipitation from 0.9% NaCl onto the film surface depended on the elemental composition of the surface layer conditioned by the thickness growth of the a-C:H:SiOx film. Based on the results of energy dispersive X-ray spectroscopy, the multiple regression equations are suggested to explain the effect of the elemental composition of the a-C:H:SiOx film on the decreased Na+ and Cl− precipitation. As a result, the a-C:H:SiOx films successfully combine good adhesion strength and rare ion precipitation and thus are rather promising for medical applications on cardiovascular stents and/or friction parts of heart pumps. 
461 |t Materials 
463 |t Vol. 15, iss. 12  |v [4239, 17 p.]  |d 2022 
610 1 |a электронный ресурс 
610 1 |a труды учёных ТПУ 
610 1 |a diamond-like nanocomposite 
610 1 |a a-C:H:SiOx film 
610 1 |a adhesion 
610 1 |a five-week biodegradation 
610 1 |a 0.9% NaCl solution 
610 1 |a алмазоподобные соединения 
610 1 |a нанокомпозиты 
610 1 |a адгезия 
701 1 |a Grenaderov  |b A. S.  |g Aleksandr Sergeevich 
701 1 |a Solovyev  |b A.  |g Andrey 
701 1 |a Oskomov  |b K. V.  |g Konstantin Vladimirovich 
701 1 |a Porokhova  |b E.  |g Ekaterina 
701 1 |a Brazovsky (Brazovskii)  |b K. S.  |c specialist in the field of electronics  |c candidate of medical Sciences, associate Professor Tomsk Polytechnic University  |f 1971-  |g Konstantin Stanislavovich  |3 (RuTPU)RU\TPU\pers\36870  |9 19899 
701 1 |a Gorokhova  |b A. V.  |g Anna Viktorovna 
701 1 |a Nasibov  |b T.  |g Temur 
701 1 |a Litvinova  |b L.  |g Larisa 
701 1 |a Khlusov  |b I. A.  |c biophysicist  |c Professor of Tomsk Polytechnic University, doctor of medical Sciences  |f 1963-  |g Igor Albertovich  |3 (RuTPU)RU\TPU\pers\34907  |9 18225 
712 0 2 |a Национальный исследовательский Томский политехнический университет  |b Исследовательская школа химических и биомедицинских технологий  |c (2017- )  |3 (RuTPU)RU\TPU\col\23537 
801 0 |a RU  |b 63413507  |c 20220706  |g RCR 
856 4 |u https://doi.org/10.3390/ma15124239 
942 |c CF