SERS platform for detection of lipids and disease markers prepared using modification of plasmonic-active gold gratings by lipophilic moieties; Sensors and Actuators B: Chemical; Vol. 265

Dades bibliogràfiques
Parent link:Sensors and Actuators B: Chemical
Vol. 265.— 2018.— [P. 182-192]
Autor corporatiu: Национальный исследовательский Томский политехнический университет Исследовательская школа химических и биомедицинских технологий
Altres autors: Guselnikova O. A. Olga Andreevna, Kalachyova E. Evgeniya, Grobonova K. Karolina, Trusova M. E. Marina Evgenievna, Barek J. Jiri, Postnikov P. S. Pavel Sergeevich, Svorcik V. Vaclav, Lyutakov O. Oleksy
Sumari:Title screen
New functional SERS platform for effective detection of lipophilic disease markers was proposed and realized. The work was aimed at the achievement of highly-reproducible SERS results obtained in shorter measuring times. The homogeneous plasmon distribution was achieved through the introduction of large area surface plasmon-polariton supported substrate with a good smearing of plasmon intensity along the working substrate area. Homogeneous distribution of targeted lipophilic molecules on the SERS surface was realized through the surface grafting with alkylaryl moieties of various carbon chain lengths via diazonium chemistry. The process of modification was followed and confirmed by XPS and Raman methods. The functionality of created SERS substrates was studied by the contact angle measurement and CVA methods. The possibility of detection of two biomedically significant molecules (squalene and beta-sitosterol) was examined. Dependence of the SERS results on the aliphatic chain lengths was tested in the terms of targeted molecules SERS intensity and reproducibility. The prepared SERS substrates were found to be suitable for sensing of squalene and beta-sitosterol at the biorelevant [mu]M concentration level.
Idioma:anglès
Publicat: 2018
Matèries:
Accés en línia:https://doi.org/10.1016/j.snb.2018.03.016
Format: Electrònic Capítol de llibre
KOHA link:https://koha.lib.tpu.ru/cgi-bin/koha/opac-detail.pl?biblionumber=667153

MARC

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200 1 |a SERS platform for detection of lipids and disease markers prepared using modification of plasmonic-active gold gratings by lipophilic moieties  |f O. A. Guselnikova, E. Kalachyova, K. Grobonova [et al.] 
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330 |a New functional SERS platform for effective detection of lipophilic disease markers was proposed and realized. The work was aimed at the achievement of highly-reproducible SERS results obtained in shorter measuring times. The homogeneous plasmon distribution was achieved through the introduction of large area surface plasmon-polariton supported substrate with a good smearing of plasmon intensity along the working substrate area. Homogeneous distribution of targeted lipophilic molecules on the SERS surface was realized through the surface grafting with alkylaryl moieties of various carbon chain lengths via diazonium chemistry. The process of modification was followed and confirmed by XPS and Raman methods. The functionality of created SERS substrates was studied by the contact angle measurement and CVA methods. The possibility of detection of two biomedically significant molecules (squalene and beta-sitosterol) was examined. Dependence of the SERS results on the aliphatic chain lengths was tested in the terms of targeted molecules SERS intensity and reproducibility. The prepared SERS substrates were found to be suitable for sensing of squalene and beta-sitosterol at the biorelevant [mu]M concentration level. 
461 |t Sensors and Actuators B: Chemical 
463 |t Vol. 265  |v [P. 182-192]  |d 2018 
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701 1 |a Guselnikova  |b O. A.  |c chemist  |c Researcher at Tomsk Polytechnic University, Candidate of Chemical Sciences  |f 1992-  |g Olga Andreevna  |3 (RuTPU)RU\TPU\pers\34478  |9 17861 
701 1 |a Kalachyova  |b E.  |c chemical engineer  |c assistant of Tomsk Polytechnic University  |f 1987-  |g Evgeniya  |3 (RuTPU)RU\TPU\pers\39642 
701 1 |a Grobonova  |b K.  |g Karolina 
701 1 |a Trusova  |b M. E.  |c organic chemist  |c Associate professor of Tomsk Polytechnic University, Candidate of chemical sciences  |f 1982-  |g Marina Evgenievna  |3 (RuTPU)RU\TPU\pers\31823  |9 15918 
701 1 |a Barek  |b J.  |g Jiri 
701 1 |a Postnikov  |b P. S.  |c organic chemist  |c Associate Professor of Tomsk Polytechnic University, Candidate of chemical sciences  |f 1984-  |g Pavel Sergeevich  |3 (RuTPU)RU\TPU\pers\31287  |9 15465 
701 1 |a Svorcik  |b V.  |g Vaclav 
701 1 |a Lyutakov  |b O.  |g Oleksy 
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