Effects of persulfate and hydrogen peroxide on oxidation of oxalate by pulsed corona discharge; Chemical Engineering Journal; Vol. 411

Dades bibliogràfiques
Parent link:Chemical Engineering Journal
Vol. 411.— 2021.— [128586, 9 p.]
Autor corporatiu: Национальный исследовательский Томский политехнический университет Инженерная школа новых производственных технологий Научно-производственная лаборатория "Чистая вода"
Altres autors: Tikker P. Priit, Dulova N. Niina, Kornev Ya. I. Yakov Ivanovich, Preys S. Sergey
Sumari:Title screen
Application of gas-phase pulsed corona discharge (PCD) to oxidation of aqueous pollutants shows unequalled energy efficiency among advanced oxidation processes (AOPs). Improved AOPs often activate extrinsic oxidants. Experimental research was undertaken into sodium persulfate and hydrogen peroxide activation by PCD in oxidation of 1.11 mM oxalate. Oxidant and target compound concentration ratios, pH, gas-liquid contact surface and pulse repetition frequency were studied as control parameters. Results implicated a beneficial effect at oxalate/persulfate molar ratios from 1:0.1 to 1:1 in acidic medium with the optimum at 1:0.5, moderate contact surface and lower frequency. However, the observed synergism of PCD/PS combination decreased with increasing the initial pH of the treated solution. Hydrogen peroxide exhibited negative or neutral impact in all media. Non-assisted PCD proved the most energy efficient approach towards water treatment at neutral and alkaline conditions.
Режим доступа: по договору с организацией-держателем ресурса
Idioma:anglès
Publicat: 2021
Matèries:
Accés en línia:https://doi.org/10.1016/j.cej.2021.128586
Format: MixedMaterials Electrònic Capítol de llibre
KOHA link:https://koha.lib.tpu.ru/cgi-bin/koha/opac-detail.pl?biblionumber=665164