An Analysis of Vibrations and Rotations in the First Hydrogen Sulfide Hexade: the 4ν2 H322S Band; Optics and Spectroscopy; Vol. 129, iss. 1

Dettagli Bibliografici
Parent link:Optics and Spectroscopy
Vol. 129, iss. 1.— 2021.— [P. 6-11]
Autore principale: Zhang Fangce
Ente Autore: Национальный исследовательский Томский политехнический университет Исследовательская школа физики высокоэнергетических процессов
Altri autori: Raspopova N. I. Natalya Ivanovna
Riassunto:Title screen
The infrared spectrum of the H2S molecule is recorded using a Bruker IFS 125HR Fourier transform spectrometer and studied in the range of 4500-5000 cm-1, in which the first hexad of bands of interacting states of the hydrogen sulfide molecule is located (in this particular case, weak band 4ν2ν2 is studied). Four hundred transitions with maximum quantum numbers of JmaxJmax = 17 and KmaxaKamax = 8 are assigned in the experimental spectrum. These transitions correspond to one hundred thirty two upper vibration-rotation energy levels. The obtained data are analyzed using Watson's model of the effective Hamiltonian. By solving the inverse spectroscopic problem, a set of twenty eight spectroscopic parameters was obtained, which reproduces the initial experimental data with a standard deviation of drmsdrms= 3.5 × 10-4 cm-1.
Режим доступа: по договору с организацией-держателем ресурса
Lingua:inglese
Pubblicazione: 2021
Soggetti:
Accesso online:https://doi.org/10.1134/S0030400X21010045
Natura: Elettronico Capitolo di libro
KOHA link:https://koha.lib.tpu.ru/cgi-bin/koha/opac-detail.pl?biblionumber=664699

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200 1 |a An Analysis of Vibrations and Rotations in the First Hydrogen Sulfide Hexade: the 4ν2 H322S Band  |f Zhang Fangce, N. I. Raspopova 
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300 |a Title screen 
320 |a [References: 16 tit.] 
330 |a The infrared spectrum of the H2S molecule is recorded using a Bruker IFS 125HR Fourier transform spectrometer and studied in the range of 4500-5000 cm-1, in which the first hexad of bands of interacting states of the hydrogen sulfide molecule is located (in this particular case, weak band 4ν2ν2 is studied). Four hundred transitions with maximum quantum numbers of JmaxJmax = 17 and KmaxaKamax = 8 are assigned in the experimental spectrum. These transitions correspond to one hundred thirty two upper vibration-rotation energy levels. The obtained data are analyzed using Watson's model of the effective Hamiltonian. By solving the inverse spectroscopic problem, a set of twenty eight spectroscopic parameters was obtained, which reproduces the initial experimental data with a standard deviation of drmsdrms= 3.5 × 10-4 cm-1. 
333 |a Режим доступа: по договору с организацией-держателем ресурса 
461 |t Optics and Spectroscopy 
463 |t Vol. 129, iss. 1  |v [P. 6-11]  |d 2021 
610 1 |a электронный ресурс 
610 1 |a труды учёных ТПУ 
610 1 |a molecular spectroscopy 
610 1 |a first hydrogen sulfide hexade 
610 1 |a vibration-rotation Hamiltonian 
610 1 |a молекулярная спектроскопия 
610 1 |a гамильтонианы 
700 0 |a Zhang Fangce  |c Chinese physicist  |c technician of Tomsk Polytechnic University  |f 1993-  |3 (RuTPU)RU\TPU\pers\42500 
701 1 |a Raspopova  |b N. I.  |c physicist  |c Associate Professor of Tomsk Polytechnic University, Candidate of Physical and Mathematical Sciences  |f 1990-  |g Natalya Ivanovna  |3 (RuTPU)RU\TPU\pers\34080  |9 17636 
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