Spectral broadening of a single Ce3+-doped garnet by chemical unit cosubstitution for near ultraviolet LED

Bibliographic Details
Parent link:Optical Materials Express
Vol. 8, iss. 12.— 2018.— [P. 3761-3769]
Corporate Authors: Национальный исследовательский Томский политехнический университет Инженерная школа новых производственных технологий Отделение материаловедения, Национальный исследовательский Томский политехнический университет Инженерная школа новых производственных технологий
Other Authors: Khan (Han) Tao, Lang Tianchun, Zhong Yang, Cao Shixiu, Peng Lingling, Yakovlev A. N. Aleksey Nikolaevich, Polisadova E. F. Elena Fyodorovna
Summary:Title screen
In this paper, the isostructural Mg3Al2Si3O12 was introduced into the Ce3+-doped yttrium aluminum garnet (Y3Al5O12) for synthesizing (Y1-xMgx)3Al2(Al1-xSix)3O12:Ce3+ (x = 0-0.6) solid solution phosphors. The co-substitution of the (Mg, Si)6+ pair for the (Y, Al)6+ pair leads to lattice shrinkage and then changes the spectral shape and width. The band peaking at ~450 nm shows a substantial broadening with the full width at half maximum increasing from 65 nm to 94 nm. The intensity of excitation spectrum (x = 0.5) at 400 nm is increased by 50% than that (x = 0). The near ultraviolet LED was fabricated with Y1.5Mg1.5Al3.5Si1.5O12:Ce3+ phosphors and a 400 nm chip and can emit strong white light. Therefore, by controlling the content of (Y, Al)6+ substituted by (Mg, Si)6+, the excitation spectrum of Ce3+-doped Y3Al5O12 can be tuned and applied for the near ultraviolet LEDs.
Language:English
Published: 2018
Subjects:
Online Access:http://earchive.tpu.ru/handle/11683/64942
https://doi.org/10.1364/OME.8.003761
Format: Electronic Book Chapter
KOHA link:https://koha.lib.tpu.ru/cgi-bin/koha/opac-detail.pl?biblionumber=659735

MARC

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200 1 |a Spectral broadening of a single Ce3+-doped garnet by chemical unit cosubstitution for near ultraviolet LED  |f Khan (Han) Tao, Lang Tianchun, Zhong Yang [et al.] 
203 |a Text  |c electronic 
300 |a Title screen 
320 |a [References: 17 tit.] 
330 |a In this paper, the isostructural Mg3Al2Si3O12 was introduced into the Ce3+-doped yttrium aluminum garnet (Y3Al5O12) for synthesizing (Y1-xMgx)3Al2(Al1-xSix)3O12:Ce3+ (x = 0-0.6) solid solution phosphors. The co-substitution of the (Mg, Si)6+ pair for the (Y, Al)6+ pair leads to lattice shrinkage and then changes the spectral shape and width. The band peaking at ~450 nm shows a substantial broadening with the full width at half maximum increasing from 65 nm to 94 nm. The intensity of excitation spectrum (x = 0.5) at 400 nm is increased by 50% than that (x = 0). The near ultraviolet LED was fabricated with Y1.5Mg1.5Al3.5Si1.5O12:Ce3+ phosphors and a 400 nm chip and can emit strong white light. Therefore, by controlling the content of (Y, Al)6+ substituted by (Mg, Si)6+, the excitation spectrum of Ce3+-doped Y3Al5O12 can be tuned and applied for the near ultraviolet LEDs. 
461 |t Optical Materials Express 
463 |t Vol. 8, iss. 12  |v [P. 3761-3769]  |d 2018 
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701 0 |a Lang Tianchun 
701 0 |a Zhong Yang  |c specialist in the field of lightning engineering  |c Associate Professor of Tomsk Polytechnic University, Ph.D  |f 1990-  |3 (RuTPU)RU\TPU\pers\39798  |9 21098 
701 0 |a Cao Shixiu 
701 0 |a Peng Lingling 
701 1 |a Yakovlev  |b A. N.  |c specialist in the field of lightning engineering  |c Vice-rector-Director of Tomsk Polytechnic University, Candidate of physical and mathematical sciences  |f 1971-  |g Aleksey Nikolaevich  |3 (RuTPU)RU\TPU\pers\31580  |9 15740 
701 1 |a Polisadova  |b E. F.  |c specialist in the field of lighting engineering  |c professor of Tomsk Polytechnic University, doctor of physical and mathematical sciences  |f 1972-  |g Elena Fyodorovna  |3 (RuTPU)RU\TPU\pers\33900  |9 17473 
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