Functional and Switchable Amphiphilic PMMA Surface Prepared by 3D Selective Modification

Bibliografske podrobnosti
Parent link:Advanced Materials Interfaces
Vol. 5, iss. 4.— 2018.— [1701182, 9 p.]
Korporativna značnica: Национальный исследовательский Томский политехнический университет Исследовательская школа химических и биомедицинских технологий (ИШХБМТ)
Drugi avtorji: Guselnikova O. A. Olga Andreevna, Postnikov P. S. Pavel Sergeevich, Sajdl P. Petr, Elashnikov R. Roman, Svorcik V. Vaclav, Lyutakov O. Oleksy
Izvleček:Title screen
The design and creation of switchable amphiphilicity on the surface of thin poly(methylmethacrylate) (PMMA) films are described. Amphiphilic properties are achieved through the 3D surface spatially selective modification using the membrane?assisted diazonium approach. Proposed technique allows simple grafting with the hydrophilic and hydrophobic compounds in the surface valleys or tops, depending on the order of modification steps. Thermally controllable hydro? and oleophilicity are achieved by the in?plane and height distinguished grafting of PMMA films with bis(trifluoromethyl)phenyl and poly(N?isopropylacrylamide) chains. Sample surface at different stages of the modification is characterized by the X?ray photoelectron spectroscopy (XPS), Fourier?transform infrared spectroscopy (FTIR), confocal microscopy, scanning electron microscopy–energy dispersive spectroscopy, and atomic force microscopy (AFM). Also the range of temperature?dependent wettability tests (with water, hexadecane, and ethyleneglycol) is performed. The temperature controlled amphiphilicity switching is proved to be fully reversible and proceeding in seconds.
Режим доступа: по договору с организацией-держателем ресурса
Jezik:angleščina
Izdano: 2018
Teme:
Online dostop:https://doi.org/10.1002/admi.201701182
Format: Elektronski Book Chapter
KOHA link:https://koha.lib.tpu.ru/cgi-bin/koha/opac-detail.pl?biblionumber=657909

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330 |a The design and creation of switchable amphiphilicity on the surface of thin poly(methylmethacrylate) (PMMA) films are described. Amphiphilic properties are achieved through the 3D surface spatially selective modification using the membrane?assisted diazonium approach. Proposed technique allows simple grafting with the hydrophilic and hydrophobic compounds in the surface valleys or tops, depending on the order of modification steps. Thermally controllable hydro? and oleophilicity are achieved by the in?plane and height distinguished grafting of PMMA films with bis(trifluoromethyl)phenyl and poly(N?isopropylacrylamide) chains. Sample surface at different stages of the modification is characterized by the X?ray photoelectron spectroscopy (XPS), Fourier?transform infrared spectroscopy (FTIR), confocal microscopy, scanning electron microscopy–energy dispersive spectroscopy, and atomic force microscopy (AFM). Also the range of temperature?dependent wettability tests (with water, hexadecane, and ethyleneglycol) is performed. The temperature controlled amphiphilicity switching is proved to be fully reversible and proceeding in seconds. 
333 |a Режим доступа: по договору с организацией-держателем ресурса 
461 |t Advanced Materials Interfaces 
463 |t Vol. 5, iss. 4  |v [1701182, 9 p.]  |d 2018 
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701 1 |a Guselnikova  |b O. A.  |c chemist  |c Researcher at Tomsk Polytechnic University, Candidate of Chemical Sciences  |f 1992-  |g Olga Andreevna  |3 (RuTPU)RU\TPU\pers\34478  |9 17861 
701 1 |a Postnikov  |b P. S.  |c organic chemist  |c Associate Professor of Tomsk Polytechnic University, Candidate of chemical sciences  |f 1984-  |g Pavel Sergeevich  |3 (RuTPU)RU\TPU\pers\31287  |9 15465 
701 1 |a Sajdl  |b P.  |g Petr 
701 1 |a Elashnikov  |b R.  |g Roman 
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