Halogenating and nitrating activity of reagents based on sodium nitrate and alkali metal halides in acetic acid

Detalles Bibliográficos
Parent link:Russian Journal of Organic Chemistry.— , 2001-
Vol. 40, iss. 7.— 2004.— [P. 917-923]
Otros Autores: Filimonov V. D. Viktor Dmitrievich, Kulmanakova Yu. Yu., Yusubov M. S. Mekhman Suleiman-Ogly (Suleimanovich), Perederina I. A., Ki-Whan Chi, Poleshchuk O. Kh. Oleg Khemovich
Sumario:Title screen
Alkali metal halides NaF, KCl, and KBr sharply enhance the nitrating activity of sodium nitrate in acetic acid with respect to 9-methylcarbazole. In the presence of KI and KBr, both nitration and halogenation of the substrate occurs, while KCl and NaF promote only the nitration process. The results may be interpreted in terms of formation of the corresponding nitryl halides XNO2 (X = F, Cl, Br, I) whose structure and reactivity were examined in the framework of the density functional theory (DFT B3LYP/3-21G*).
Режим доступа: по договору с организацией-держателем ресурса
Lenguaje:inglés
Publicado: 2004
Materias:
Acceso en línea:http://dx.doi.org/10.1023/B:RUJO.0000045178.33131.c2
Formato: Electrónico Capítulo de libro
KOHA link:https://koha.lib.tpu.ru/cgi-bin/koha/opac-detail.pl?biblionumber=647610

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200 1 |a Halogenating and nitrating activity of reagents based on sodium nitrate and alkali metal halides in acetic acid  |f V. D. Filimonov [et al.] 
203 |a Text  |c electronic 
300 |a Title screen 
320 |a [References: p. 923 (22 tit.)] 
330 |a Alkali metal halides NaF, KCl, and KBr sharply enhance the nitrating activity of sodium nitrate in acetic acid with respect to 9-methylcarbazole. In the presence of KI and KBr, both nitration and halogenation of the substrate occurs, while KCl and NaF promote only the nitration process. The results may be interpreted in terms of formation of the corresponding nitryl halides XNO2 (X = F, Cl, Br, I) whose structure and reactivity were examined in the framework of the density functional theory (DFT B3LYP/3-21G*). 
333 |a Режим доступа: по договору с организацией-держателем ресурса 
461 |t Russian Journal of Organic Chemistry  |d 2001- 
463 |t Vol. 40, iss. 7  |v [P. 917-923]  |d 2004 
610 1 |a электронный ресурс 
610 1 |a труды учёных ТПУ 
610 1 |a reagents 
610 1 |a acetic acid 
610 1 |a alkali metals 
610 1 |a реагенты 
610 1 |a щелочные металлы 
610 1 |a уксусная кислота 
701 1 |a Filimonov  |b V. D.  |c Russian chemist  |c Professor of the TPU  |f 1945-  |g Viktor Dmitrievich  |3 (RuTPU)RU\TPU\pers\26423  |9 12127 
701 1 |a Kulmanakova  |b Yu. Yu. 
701 1 |a Yusubov  |b M. S.  |c chemist  |c Professor of Tomsk Polytechnic University, Doctor of chemical sciences  |f 1961-  |g Mekhman Suleiman-Ogly (Suleimanovich)  |3 (RuTPU)RU\TPU\pers\31833  |9 15928 
701 1 |a Perederina  |b I. A. 
701 1 |a Ki-Whan Chi 
701 1 |a Poleshchuk  |b O. Kh.  |c chemist  |c Professor-consultant of Yurga technological Institute of Tomsk Polytechnic University, Doctor of chemical sciences  |f 1947-  |g Oleg Khemovich  |3 (RuTPU)RU\TPU\pers\31825  |9 15920 
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