CO[2] Sequestration by Natural Zeolite for Greenhouse Effect Control

Detaylı Bibliyografya
Parent link:Procedia Chemistry
Vol. 15 : Chemistry and Chemical Engineering in XXI century (CCE 2015).— 2015.— [P. 33-41]
Müşterek Yazar: Национальный исследовательский Томский политехнический университет (ТПУ) Институт природных ресурсов (ИПР) Кафедра технологии органических веществ и полимерных материалов (ТОВПМ)
Diğer Yazarlar: Hernandez M. A. Miguel Angel, Pestryakov A. N. Aleksey Nikolaevich, Portillo R. Roberto, Salgado M. A. Martha, Rojas F. Fernando, Rubio E. Efrain, Ruiz S. Sinuhe, Petranovskii V. Vitalii
Özet:Title screen
This paper describes the adsorption of CO[2] on pores in natural erionite exchanged with aqueous solutions of Na{+}, Mg{2+}, and Ca{2+} salts at different concentrations, variable time and temperature of treatment. Experimental data of CO[2] adsorption were treated by the Freundlich and Langmuir equations. Complementarily were evaluated standard adsorption energies and the degree of interaction of the gas with the zeolite; the evolution of isosteric heats of adsorption was analyzed. The exchange with Na{+} favors the creation of emergent pores thus causing an increase of the adsorption capacity for CO[2]. The presence of Na{+} at micropore entrances causes an increased adsorption into the nanocavities and on the external area of the ion-exchanged zeolites. The development of nanopores in erionite was evaluated through the Barrett-Joyner-Halenda and NLDFT methods. Depending on the conditions of the exchange treatment, Na{+} was found to be most favorable, well distributed, and accessible for N[2] adsorption.
Режим доступа: по договору с организацией-держателем ресурса
Dil:İngilizce
Baskı/Yayın Bilgisi: 2015
Konular:
Online Erişim:http://dx.doi.org/10.1016/j.proche.2015.10.006
http://earchive.tpu.ru/handle/11683/15082
Materyal Türü: Elektronik Kitap Bölümü
KOHA link:https://koha.lib.tpu.ru/cgi-bin/koha/opac-detail.pl?biblionumber=645299

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330 |a This paper describes the adsorption of CO[2] on pores in natural erionite exchanged with aqueous solutions of Na{+}, Mg{2+}, and Ca{2+} salts at different concentrations, variable time and temperature of treatment. Experimental data of CO[2] adsorption were treated by the Freundlich and Langmuir equations. Complementarily were evaluated standard adsorption energies and the degree of interaction of the gas with the zeolite; the evolution of isosteric heats of adsorption was analyzed. The exchange with Na{+} favors the creation of emergent pores thus causing an increase of the adsorption capacity for CO[2]. The presence of Na{+} at micropore entrances causes an increased adsorption into the nanocavities and on the external area of the ion-exchanged zeolites. The development of nanopores in erionite was evaluated through the Barrett-Joyner-Halenda and NLDFT methods. Depending on the conditions of the exchange treatment, Na{+} was found to be most favorable, well distributed, and accessible for N[2] adsorption. 
333 |a Режим доступа: по договору с организацией-держателем ресурса 
461 0 |0 (RuTPU)RU\TPU\network\3889  |t Procedia Chemistry 
463 0 |0 (RuTPU)RU\TPU\network\10324  |t Vol. 15 : Chemistry and Chemical Engineering in XXI century (CCE 2015)  |o XVI International Scientific Conference dedicated to Professor L.P. Kulyov, 25-29 May 2015, Tomsk, Russia  |f National Research Tomsk Polytechnic University (TPU) ; ed. E. I. Korotkova  |v [P. 33-41]  |d 2015 
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