Characterization of a Novel Dioxomolybdenum Complex by Cyclic Voltammetry

Dettagli Bibliografici
Parent link:Analytical Letters
Vol. 48, iss. 15.— 2015.— [P. 2369-2379]
Ente Autore: Национальный исследовательский Томский политехнический университет (ТПУ) Институт природных ресурсов (ИПР) Кафедра технологии органических веществ и полимерных материалов (ТОВПМ)
Altri autori: Knittl E. T. Esther Theresa, Rusakov D. A. Dmitry Aleksandrovich, Korotkova E. I. Elena Ivanovna, Dorozhko E. V. Elena Vladimirovna, Voronova O. A. Olesya Aleksandrovna, Plotnikov E. V. Evgeny Vladimirovich, Topaloglu-Sozuer I. Isil, Linert W. Wolfgang
Riassunto:Title screen
Metalloenzymes that carry a pterin-based molybdenum cofactor in their center catalyze numerous reactions in the human body and play a crucial role in its metabolism. Specifically, these enzymes promote redox reactions and oxygen transport in the body. Their absence may cause many problems leading to disability or even death in early childhood. Therefore, model compounds need to be synthesized and analyzed to investigate the reactivity, redox potential, and geometry of these cofactors. This study focused on electrode processes and determined the redox potentials of the new bis-(4-mercapto-5-(p-tolyl)-3H-1,2-dithiole-3-thione)-dioxomolybdenum complex by cyclic voltammetry. The 4-mercapto-5-(p-tolyl)-3H-1,2-dithiole-3-thione ligand underwent irreversible oxidation and reduction at thiol and thione functional groups. The new dioxomolybdenum complex showed a quasi-reversible two-stage electrode process.
Режим доступа: по договору с организацией-держателем ресурса
Lingua:inglese
Pubblicazione: 2015
Soggetti:
Accesso online:http://dx.doi.org/10.1080/00032719.2015.1038555
Natura: Elettronico Capitolo di libro
KOHA link:https://koha.lib.tpu.ru/cgi-bin/koha/opac-detail.pl?biblionumber=644197

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200 1 |a Characterization of a Novel Dioxomolybdenum Complex by Cyclic Voltammetry  |f E. T. Knittl [et al.] 
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300 |a Title screen 
330 |a Metalloenzymes that carry a pterin-based molybdenum cofactor in their center catalyze numerous reactions in the human body and play a crucial role in its metabolism. Specifically, these enzymes promote redox reactions and oxygen transport in the body. Their absence may cause many problems leading to disability or even death in early childhood. Therefore, model compounds need to be synthesized and analyzed to investigate the reactivity, redox potential, and geometry of these cofactors. This study focused on electrode processes and determined the redox potentials of the new bis-(4-mercapto-5-(p-tolyl)-3H-1,2-dithiole-3-thione)-dioxomolybdenum complex by cyclic voltammetry. The 4-mercapto-5-(p-tolyl)-3H-1,2-dithiole-3-thione ligand underwent irreversible oxidation and reduction at thiol and thione functional groups. The new dioxomolybdenum complex showed a quasi-reversible two-stage electrode process. 
333 |a Режим доступа: по договору с организацией-держателем ресурса 
461 |t Analytical Letters 
463 |t Vol. 48, iss. 15  |v [P. 2369-2379]  |d 2015 
610 1 |a электронный ресурс 
610 1 |a труды учёных ТПУ 
610 1 |a циклическая вольтамперометрия 
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610 1 |a окислительно-восстановительные свойства 
701 1 |a Knittl  |b E. T.  |g Esther Theresa 
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701 1 |a Korotkova  |b E. I.  |c chemist  |c Professor of Tomsk Polytechnic University, Doctor of chemical science  |f 1965-  |g Elena Ivanovna  |3 (RuTPU)RU\TPU\pers\31278  |9 15456 
701 1 |a Dorozhko  |b E. V.  |c chemist  |c Engineer of Tomsk Polytechnic University  |f 1979-  |g Elena Vladimirovna  |3 (RuTPU)RU\TPU\pers\32174  |9 16175 
701 1 |a Voronova  |b O. A.  |c chemist  |c Assistant of Tomsk Polytechnic University, Candidate of chemical sciences  |f 1979-  |g Olesya Aleksandrovna  |3 (RuTPU)RU\TPU\pers\32169  |9 16170 
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