Vanadium Oxide Catalysts on Structured Microfiber Supports for the Selective Oxidation of Hydrogen Sulfide

Détails bibliographiques
Parent link:Catalysis in Industry: Scientific Journal
Vol. 7, iss. 2.— 2015.— [P. 155-160]
Collectivité auteur: Национальный исследовательский Томский политехнический университет (ТПУ) Институт природных ресурсов (ИПР) Кафедра химической технологии топлива и химической кибернетики (ХТТ)
Autres auteurs: Mikenin P. E., Tsyrulnikov P. G., Kotolevichb Y. S., Kravtsov А. V. Anatoly Vasilyevich, Ivanchina E. D. Emilia Dmitrievna, Zagoruiko A. N. Andrey Nikolaevich
Résumé:Title screen
Vanadium(V) oxide catalysts for the selective oxidation of hydrogen sulfide to sulfur on a nonporous glassfiber support with a surface layer of a porous secondary support (SiO2) are studied. The catalystsare obtained by means of pulsed surface thermosynthesis. Such catalysts are shown to have high activity andacceptable selectivity in the industrially important region of temperatures below 200°C. A glassfiber catalystcontaining vanadium oxide (10.3 wt % of vanadium) in particular ensures the complete conversion of H2S ata temperature of 175°C and a reaction mixture hourly space velocity (RMHSV) of 1 cm3/(gcat s) with a sulfuryield of 67%; this is at least 1.35 times higher than for the traditional iron oxide catalyst. Using a structuredglassfiber woven support effectively minimizes diffusion resistance and greatly simplifies the scaleup of processes based on such catalysts. Such catalysts can be used for the cleansing of tail gases from Claus units andin other processes based on the selective oxidation of H2S.
Режим доступа: по договору с организацией-держателем ресурса
Langue:anglais
Publié: 2015
Sujets:
Accès en ligne:http://dx.doi.org/10.1134/S2070050415020075
Format: Électronique Chapitre de livre
KOHA link:https://koha.lib.tpu.ru/cgi-bin/koha/opac-detail.pl?biblionumber=643123

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200 1 |a Vanadium Oxide Catalysts on Structured Microfiber Supports for the Selective Oxidation of Hydrogen Sulfide  |f P. E. Mikenin [et al.] 
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300 |a Title screen 
320 |a [References: p. 159-160 (25 tit.)] 
330 |a Vanadium(V) oxide catalysts for the selective oxidation of hydrogen sulfide to sulfur on a nonporous glassfiber support with a surface layer of a porous secondary support (SiO2) are studied. The catalystsare obtained by means of pulsed surface thermosynthesis. Such catalysts are shown to have high activity andacceptable selectivity in the industrially important region of temperatures below 200°C. A glassfiber catalystcontaining vanadium oxide (10.3 wt % of vanadium) in particular ensures the complete conversion of H2S ata temperature of 175°C and a reaction mixture hourly space velocity (RMHSV) of 1 cm3/(gcat s) with a sulfuryield of 67%; this is at least 1.35 times higher than for the traditional iron oxide catalyst. Using a structuredglassfiber woven support effectively minimizes diffusion resistance and greatly simplifies the scaleup of processes based on such catalysts. Such catalysts can be used for the cleansing of tail gases from Claus units andin other processes based on the selective oxidation of H2S. 
333 |a Режим доступа: по договору с организацией-держателем ресурса 
461 |t Catalysis in Industry  |o Scientific Journal 
463 |t Vol. 7, iss. 2  |v [P. 155-160]  |d 2015 
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701 1 |a Kotolevichb  |b Y. S. 
701 1 |a Kravtsov  |b А. V.  |c Russian chemical engineer  |c Consulting Professor, Doctor of Technical Sciences (DSc)  |f 1938-2012  |g Anatoly Vasilyevich  |3 (RuTPU)RU\TPU\pers\29428 
701 1 |a Ivanchina  |b E. D.  |c chemist  |c Professor of Tomsk Polytechnic University, Doctor of technical sciences  |f 1951-  |g Emilia Dmitrievna  |3 (RuTPU)RU\TPU\pers\31274 
701 1 |a Zagoruiko  |b A. N.  |c Chemical Engineer  |c Professor of Tomsk Polytechnic University, Doctor of technical sciences  |f 1962-  |g Andrey Nikolaevich  |3 (RuTPU)RU\TPU\pers\33191 
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